Which Alumilite are you using? If you are using Alumilite Clear, I doubt you will find much in a casting resin that is harder. Folks say that Alumilite Clear is not as hard as acrylic but the technical properties does not back this up. Acrylic typically has a shore D hardness of 80 while Alumilite Clear is also 80D. Now, if you are using Alumilite White, it is 72D which is quite a bit softer.
If you are going solely by feel of turning, then other tech properties come into play such as elongation which is a measurement of how much it will stretch before it breaks. Alumilite has a high elongation which is what makes it turn like butter. Acrylics typically have a very small elongation which makes them more brittle.